This thesis presents an account of experimental and numerical investigations of two quantum systems whose respective classical analogues are chaotic. These are the delta-kicked rotor, a paradigm in classical chaos theory, and the novel delta-kicked accelerator, created by application of a constant external acceleration or torque to the rotor. The experimental realisation of these systems has been achieved by the exposure of laser-cooled caesium atoms to approximate delta-kicks from a pulsed, high-intensity, vertical standing wave of laser light. Gravity’s effect on the atoms can be controlled by appropriate shifting of the profile of the standing wave. Numerical simulations of the systems are based on a diffractive model of the potential’s effect. Each system’s dynamics are characterised by the final form of the momentum distribution and the dependence of the atoms’ mean kinetic energy on the number and time period of the delta-kicks. The phenomena of dynamical localisation and quantum resonances in the delta-kicked rotor, which have no counterparts in the system’s classical analogue, are observed and investigated. Similar experiments on the delta-kicked accelerator reveal the striking phenomenon of the quantum accelerator mode, in which a large momentum is transferred to a substantial fraction of the atomic ensemble. This feature, absent in the system’s classical analogue, is characterised and an analytic explanation is presented. The effect on each quantum system of decoherence, introduced through spontaneous emission in the atoms, is examined and comparison is made with the results of classical simulations. While having little effect on the classical systems, the level of decoherence used is found to degrade quantum signatures of behaviour. Classical-like behaviour is, to some extent, restored, although significant quantum features remain. Possible applications of the quantum accelerator mode are discussed. These include use as a tool in atom optics and interferometry, a technique for measuring gravity, and a method of preparing atoms in a particular region of phase space. This may allow measurement of quantum phase space stability, and hence investigation of quantum chaos and quantum-classical correspondence.